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Some to consider :
Predator 1 + 2 - Alan Silvestri I think did this, extremely atmospheric and fits perfectly with the action.
Terminator 2 - Superb soundtrack, adds to the whole atmosphere and sounds great cranked up to the max
Lock Stock - A lot of the music on this film is by famous artists, but the bits that aren't included on the soundtrack CD are very good
Escape from new York - Old skool film. John Carpenter films always have superb music, very much in the style that was common at the time (early 80s) Also, 'the thing' had some incredibly eerie music.
Aliens - nuff said, great stuff
Makes me feel like a gangster
Regarding some of the other stuff mentioned so far in this thread: Alan Silvestri did both the Predator and Back To The Future scores, Emiliana Torrini has an album worth getting called Love In The Time Of Science and to spookily link this with another post the album was co-written and produced by Roland Orzabal who was in Tears For Fears who appear (and are covered) on the Donnie Darko soundtrack!
> Back To The Future.
This is my second favourite. Great for playing flying games too. :)
Halloween
The Exorcist
The origianl Planet of the Apes
> Goo Goo Dolls - Iris or Human Traffic - Music is the drug
Iris is from City of Angels with Nicholas Cage and Meg Ryan