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"Music is my mistress, and she shall play second fiddle to none". - Duke Ellington
Although some of the most memorable tunes have come from Mario games and the brilliant Banjo Kazzoie games, they seriously stay in your head, damn catchy, even today I can remember the tune to Click Clock Wood.
k, on a more serious note. Probably Mario 64 (water level music), or Donkey Kong Country (mainly water level music again)!
Final Fantasy normally has pretty darn good music too. A Zelda OOT's soundtrack was pretty sweet to!
:)