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It really is excellent, the best online gaming experience there is. It's very reliable and with almost a million users getting a match with someone is fairly easy.
There are a whole bunch of decent Live titles, however if you were to check the Big SR Live Sheet [URL]http://members.lycos.co.uk/notoriousbiggles/[/URL] then you'd be able to see what the most popular games are. Currently Rainbow Six 3, Project Gotham Racing 2 and Splinter Cell: Pandora Tomorrow are the most popular.
I can highly recommend Rainbow Six 3 and PGR2, along with Crimson Skies, ESPN NHL Hockey and Top Spin. XIII has a great single player but I have yet to play it on Live.
When you get Live, add your gamertag and Live games (online multiplayer ones only please, i.e. not KOTOR or Ninja Gaiden which don't have online multiplayer) to the Xbox Live Definative Thread. It's a big thread with around 500 replies in it. Then I'll add you to the Big Sheet itself. Then you can die happy.
Perhaps when I get my xbox we'll be able to play with 4 users